采用溶胶-凝胶法制备了3种不同钡锶物质的量比的Ba1-xSrxAl2Si2O8 (BSAS)体系粉体材料,其钡、锶物质的量比分别为1∶0、0.75∶0.25、0∶1.将烧结得到的BSAS块体材料表面喷涂(8.5±0.2)mg/cm2的Na2SO4后,置于1000℃空气环境中进行熔盐腐蚀实验,研究其抗熔盐腐蚀性能.根据样品质量随腐蚀时间的变化,结合X射线衍射(XRD)和扫描电镜形貌分析(SEM)等结果,揭示其抗熔盐腐蚀机理.结果表明,B0.75 S0.25AS腐蚀100h后质量变化最小,XRD分析其成分未发生明显变化,说明B0.75S0.25AS在1000℃时的抗熔盐腐蚀性能优于其它物质的量比的BSAS材料.
参考文献
[1] | 张立同,成来飞,徐永东.新型碳化硅陶瓷基复合材料的研究进展[J].航空制造技术,2003(01):24-32. |
[2] | F. A. Christin .A Global Approach to Fiber nD Architectures and Self-Sealing Matrices: From Research to Production[J].International journal of applied ceramic technology,2005(2):97-104. |
[3] | Kimmel J;Miriyala N;Price J et al.Evaluation of CFCC liners with EBC after testing in a gas turbine[J].Journal of the European Ceramic Society,2002,22(14-15):2769. |
[4] | Jacobson NS.;Opila EJ.;Fox DS. .High temperature oxidation of ceramic matrix composites[J].Pure and Applied Chemistry,1998(2):493-500. |
[5] | Elizabeth J.Opila;Dennis S.Fox;Nathan S.Jacobson .Mass spectrometric identification of Si-O-H(g) species from the reaction of silica with water vapor at atmospheric pressure[J].Journal of the American Ceramic Society,1997(4):1009-1012. |
[6] | Jacobson N S .Corrosion of silicon-based ceramics in combustion environments[J].Journal of the American Ceramic Society,1993,76(01):3. |
[7] | Jacobson N S;Smialek J L .Hot corrosion of sintered a-SiC at 1000℃[J].Journal of the American Ceramic Society,1985,68(08):432. |
[8] | Jacobson N S .Kinetics and mechanism of corrosion of SiC by molten salts[J].Journal of the American Ceramic Society,2005,69(01):74. |
[9] | Tressler R E;Meiser M D;Yonushonis T .Molten salt corrosion of SiC and Si3N1 ceramics[J].Journal of the American Ceramic Society,1976,59(5-6):278. |
[10] | Karren L. More;Peter F. Tortorelli;Larry R. Walker .High-Temperature Stability of SiC-Based Composites in High-Water-Vapor-Pressure Environments[J].Journal of the American Ceramic Society,2003(8):1272-1281. |
[11] | Wu Y H;Cheng L F;Wang YG et al.Fabrication and characterization of corrosion resistance on BaO-Al2O3-SiO2 environmental barrier coatings[J].Journal of the Chinese Ceramic Society,2009,37(08):1299. |
[12] | Wang Y G;Wu Yahui;Cheng L F et al.Hot corrosion behavior of BAS coated C/SiC composites at 900 ℃[J].Journal of the American Ceramic Society,2010,93(01):204. |
[13] | Wang Y G;Fei W;Fan Y et al.Silicoaluminum carbonitride ceramic resistance to oxidation/corrosion in water vapor[J].Journal of Materials Research,2006,21(07):1625. |
[14] | Liu Limeng;Ye Feng;Zhang Haijiao .Celsian formation in Si_3N_4-Ba_(0.75)Sr_(0.25)Si_2Al_2O_8 composites[J].Scripta materialia,2009(6):463-466. |
[15] | Corrosion of barium aluminosilicates by water-vapour: An investigation from first principles[J].Corrosion Science: The Journal on Environmental Degradation of Materials and its Control,2009(9):2126. |
[16] | Kang N. Lee;Dennis S. Fox;Jeffrey I. Eldridge .Upper Temperature Limit of Environmental Barrier Coatings Based on Mullite and BSAS[J].Journal of the American Ceramic Society,2003(8):1299-1306. |
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