Lead-free piezoelectric ceramics (Na0.5K0.5-xLix)NbO3 (x=0.057–0.066) were synthesized by an ordinary sintering technique. Substituting Li for K can lead to structural distortion, which improves the Curie temperature (TC) greatly. By adding appropriate LiNbO3 content, piezoelectric constant d33 values reach 202–212 pC/N. Electromechanical coefficients of the planar mode reach 44.4%–46.8%. The dielectric loss is below 2.6%, which is much lower than reported (about 50%). The TC of (Na0.5K0.5-xLix)NbO3 (x=0.057–0.066) is in the range of 490–510oC, at least 70oC higher than that of pure (Na0.5K0.5)NbO3 ceramics. The results show that (Na0.5K0.5-xLix)NbO3 ceramic is a kind of good lead-free high-temperature piezoelectric material.
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