From the high-order perturbation formulas of spin Hamiltonian parameters based on the two spin-orbit coupling parameter model, the spin Hamiltonian parameters (g factor g(parallel to), g(perpendicular to) and zero-field splitting D) of the trigonal Co2+ center (which is assigned to a Co2+-S pair defect center) in ZnS0.001Se0.999 mixed crystal are calculated. The calculated results are comparable with the observed values, suggesting that the above assignment is suitable. (c) 2005 Elsevier B.V. All rights reserved.
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