通过溶胶-凝胶的方法,制备了La0.6Sr0.15 Na0.1□0.15MnO3与微量Ag的掺杂样品(掺杂量为x=0.000、x=0.016、x=0.040、x=0.100).测量其相结构和电榆运性质.掺杂后,x=0.016样品呈单相性;而x=0.040、x=0.100样品呈现锰氧化物与Ag的二相复合结构.掺杂样品的电阻率升高;本征磁电阻值降低.同时,由于微量Ag的掺杂,使x=0.040、x=0.100样品的自旋相关的隧道磁电阻得到加强,从而表现出了很好的磁电阻温度稳定性能:在207~286K的温度范围内,x=0.040样品的MR保持在5.08%±0.20%;在205~272 K的温度范围内,x=0.100样品的MR保持在5.00%±0.33%.
参考文献
[1] | Ziese M. .Extrinsic magnetotransport phenomena in ferromagnetic oxides [Review][J].Reports on Progress in Physics,2002(2):143-249. |
[2] | Kou Zhi-Qi,Di Nai-Li,Ma Xiao,Li Qing-An,Cheng Zhao-Hua.Enhancement of "intrinsic" magnetoresistance ratio and activation energy of La0.67Ca0.33MnO3 single crystals by Fe doping[J].中国物理(英文版),2005(08):1653-1656. |
[3] | PENG Zhensheng,WANG Guiying,TANG Yonggang,LIU Peng,NIU Xiaofei.Enhancement of room-temperature magnetoresistance in La_(0.5)Sm_(0.2)Sr_(0.3)MnO_3/(Ag_2O)_(x/2)[J].稀有金属(英文版),2010(01):45-49. |
[4] | SONG Qixiang,NIU Xiaofei,WANG Guiying,TANG Yonggang,CAI Zhirang,PENG Zhensheng.Enhancement of room-temperature magnetoresistance in La_(0.6)Dy_(0.1)Sr_(0.3)MnO_3/Ag_x[J].稀有金属(英文版),2010(02):126-131. |
[5] | G. D. Tang;D. L. Hou;Z. Z. Li;X. Zhao;W. H. Qi;S. P. Liu;F. W. Zhao .Influence of cohesive energy on unit cell volume of perovskite manganites La_(1-x)M_(x)MnO_(3)[J].Applied physics letters,2006(26):261919-1-261919-3-0. |
[6] | 赵福伟,唐贵德.La_(0.60)Sr_(0.40-x)K_xMnO_3系列材料的磁电阻效应[J].材料科学与工程学报,2012(03):468-472. |
[7] | 王桂英,杨刚,郭焕银,毛强,叶吾梅,彭振生.Cr替代Mn对La0.4Ca0.6MnO3磁性质的影响[J].无机材料学报,2011(04):411-416. |
[8] | Wang XL.;Liu HK.;Ionescu M.;Zeimetz B.;Dou SX. .Large low-field magnetoresistance over a wide temperature range induced by weak-link grain boundaries in La0.7Ca0.3MnO3[J].Applied physics letters,1998(3):396-398. |
[9] | 王桂英,彭振生,唐永刚,刘鹏,牛晓飞.La_(0.5)Sm_(0.2)Sr_(0.3)MnO_3/Ag_x二相复合体的结构及磁电阻[J].稀有金属,2010(02):210-214. |
[10] | 张炯,魏立国,张蕾,李定国,熊永红,熊曹水.Ag掺杂对La0.7Ca0.2Sr0.1MnO3室温磁电阻效应的增强[J].低温物理学报,2007(02):86-89. |
[11] | 刘力虎,唐贵德,聂向富.La0.9Sr0.1MnO3/Fe2O3复合体系的异常磁电阻效应[J].功能材料,2006(03):370-371. |
[12] | Tang V;Zhang S Y et al.Giant magnetoresistance of bulk polycrystalline La.833Na0.167 MnO with Ag2O addition[J].Journal of Alloys and Compounds,2003,353(1-2):91. |
[13] | Roy S;Guo Y Q;Venkatesh S et al.Interplay of structure and transport properties of sodium-doped lanthanum manganite[J].Journal of Physics:Condensed Matter,2001,13(42):9547. |
[14] | 原晓波,刘宜华,黄宝歆,王成建,梅良模.La0.67Ba0.33MnO3中Ag的掺杂效应[J].功能材料,2005(01):32-34. |
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