Multilayer oxides of SrNb0.1Ti0.9O3/La0.8Sr0.2MnO3/SrTiO3 have been grown by computer-controlled laser molecular beam epitaxy and characterized by transmission electron microscopy. Electron microdiffractions and high-resolution imaging reveal that the as-prepared thin film of La0.8Sr0.2MnO3 with thickness of 200 nm is epitaxially grown on the SrTiO3(001) substrate and the SrNb0.1Ti0.9O3 With thickness of 250 nm epitaxially on the as-received La0.8Sr0.2MnO3 film. The microstructures in the La0.8Sr0.2MnO3 film are clarified in terms of the oriented rnicrodomains. In contrast, microstructures in SNTO are featured by the fort-nation of superstructures due to charge ordering. Crystallographic relationships of these domains are discussed on the basis of an orthorhombic cell and rationalized by theoretical calculations based on a geometrical model.
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