垃圾填埋场渗滤液所含物质种类繁多，理化特性复杂，且随填埋时间等条件而变化。本文综合分析了垃圾渗滤液溶解性有机质的组成特征、结构特征及随年代变化特征。针对垃圾渗滤液难降解有机质的特性而研发的处理技术包括物化法、高级氧化法和微电解法等，并在实际工程中得到应用。随着越来越严格的渗滤液排放要求，溶解性有机质的去除应充分考虑投资的经济、运行的稳定性和可靠性。
There are a wide variety of substances with complex physicochemical properties in leachate from the landfill sites, and they change with conditions such as filling time. This paper reviews the composition of dissolved organic matter in landfill leachate characteristics, structure and variation with age. Several landfill leachate treatment methods have been developed to remove refractory compounds from leachate, including phsico?chemical process, advanced oxidation process, micro?electrolysis process and so on. Most of these methods have been applied in actual projects. To meet the tougher discharge standards of leachate, investment efficiency, operation stability and reliability should be adequately considered during the removal process of dissolved organic matter.
参考文献
| [1] | Kjeldsen P,Morton A B,Alix P R,et al .Present and long-term composition of MSW landfill leachate:A review[J].Critical Reviews in Environmental Science and Technology,2002,32 |
| [2] | 张彩香 .垃圾渗滤液中溶解有机质与内分泌干扰物相互作用研究[D].中国地质大学(武汉),2007. |
| [3] | Kang K,Shinb H S,Park H .Characterization of humic substances present in landfill leachates with different landfill ages and its implications[J].Water Research,2002,36 |
| [4] | He P J,Xue J F,Shao L M,et al .Dissolved organic matter(DOM)in recycled leachate of bioreactor landfill[J].Water Research,2006,40 |
| [5] | 张文义 .微波辅助过二硫酸盐对渗滤液中腐殖酸的降解研究[D].中国海洋大学,2011. |
| [6] | 刘可.城市生活垃圾渗滤液特性分析及厌氧生物处理研究[D].西安:西安建筑科技大学硕士学位论文,2004 |
| [7] | 楼紫阳,赵由才,柴晓利,牛冬杰.渗滤液中胶粒的梯度分离[J].环境科学学报,2004(01):165-167. |
| [8] | 陈少华,刘俊新.垃圾渗滤液中有机物分子量的分布及在MBR系统中的变化[J].环境化学,2005(02):153-157. |
| [9] | Steelink C.Implications of elemental characteristics of humic substances.Humic substances in soil,sediment,and water[M].New York:Wiley,1985:457-476 |
| [10] | Huo S L,Xi B D,Yu H C,et al .Characteristics of disovled organic matter (DOM)in leachate with different landfill ages[J].Journal of Environmental Science,2008,20 |
| [11] | 贾陈忠,王焰新,张彩香,秦巧燕.垃圾渗滤液中溶解性有机物组分的三维荧光特性[J].光谱学与光谱分析,2012(06):1575-1579. |
| [12] | Christensen J B,Jensen D L,Gron Christian,et al .Charaterization of the dissolved organic carbon in landfill leachate-polluted groundwater[J].Water Research,1998,32 |
| [13] | Qi G X,Yue D B,Nie Y F .Characterization of humic substances in bio-treated municipal solid waste landfill leachate[J].Frontiers of Environmental Science & Engineering,2012,6 |
| [14] | 赵庆良,卜琳.生化-物化法处理渗滤液溶解性有机物光谱特征[J].哈尔滨商业大学学报（自然科学版）,2011(03):292-295,303. |
| [15] | Castagnoli O,Musmeci L,Zavattiero E,et al .Humic substances and humification rate in a municipal refuse disposal of in a landfill[J].Water,1990,53 |
| [16] | Fan H J,Shu H Y,Yang H S,et al .Characteristics of landfill leachates in central Taiwan[J].Science of the Total Environment,2006,361 |
| [17] | Chian E S K,DeWalle F B .Characterization of soluble organic matter in leachate[J].Environmental Science and Technology,1977,11 |
| [18] | Calace N,Liberatori A,Petronio B M,et al .Characteristics of different molecular weight fractions of organic matter in landfill leachate and their role in soil sorption of heavy metals[J].Environmental Pollution,2001,113 |
| [19] | Croue J P,Benedetti M F,Violleau D,et al .Characterization and copper binding of humic and nonhumic organic matter isolated from the South Platte River.Evidence for the presence of nitrogenous binding site[J].Environmental Science and Technology,2003,37 |
| [20] | Tatsi A A,Zouboulis A I,Matis K A,et al .Coagulation-flocculation pretreatment of sanitary landfill leachates[J].Chemosphere,2003,53 |
| [21] | Liu X,Li X M,Yang Q,et al .Landfill leachate pretreatment by coagulation-flocculation process using iron-based coagulants:Optimization by response surface methodology[J].Chemical Engineering Journal,2012,200 |
| [22] | 薛俊峰,何品晶,邵立明,李国建.渗滤液循环回灌出水在混凝处理中的去除特性[J].环境污染与防治,2005(03):164-167. |
| [23] | 刘智萍,方芳,ABDULHUSSAIN A Abbas,郭劲松,姜佩言.高DOM渗滤液厌氧-好氧-混凝处理工艺[J].环境科学研究,2010(08):1081-1085. |
| [24] | 朱永强,孙力平,王少坡,王爱琴.混凝对垃圾渗滤液中腐殖质的去除特性[J].工业用水与废水,2011(02):22-25. |
| [25] | Dennett K E,Amirtharajah A,Moran T F,et al .Coagulation:Its effect on organic matter[J].American Water Works Association Journal,1996,88 |
| [26] | O′Melia C R,Becker W C,Au K K .Removal of humic substances by coagulation[J].Water Science and Technology,1999,40 |
| [27] | Bouwer E J,Crowe P B .Biological processes in drinking water treatment[J].American Water Works Association Journal,1988,80 |
| [28] | Ma H Z,Allen H E,Yin Y J .Characterization of isolated fractions of dissolved organic matter from natural waters and wastewater effluent[J].Water Research,2001,35 |
| [29] | 韩芸,杨永哲,刘可,王志盈.垃圾渗滤液及处理出水的有机物MW分布[J].中国给水排水,2006(01):88-91. |
| [30] | McCreary J J,Snoeyink V L .Characterization and activated carbon adsorption of several humic substances[J].Water Research,1980,14 |
| [31] | Semmens M J.Optimizing coagulation-adsorption for haloform and total organic carbon reduction.USEPA project summary EPA 600/52-83-042[R].Watshington D C:USEPA,1983 |
| [32] | 诸毅,岳东北,许玉东,聂永丰.膜分离腐殖酸前后晚期渗沥液的活性炭吸附特性研究[J].环境卫生工程,2007(03):25-28. |
| [33] | Kurniawan T A,Lo W H,Chan G Y S .radicals-catalyzed oxidation reactions for degradation of recalcitrant compounds from landfill leachate[J].Chemical Engineering Journal,2006,125 |
| [34] | 谭磊,王宝山.高级氧化技术处理垃圾渗滤液的研究进展[J].环境科学与管理,2009(04):87-93. |
| [35] | 朱兆连,孙敏,杨峰,王海玲,徐炎华,李爱民.微电解-Fenton氧化法去除垃圾渗滤液中有机物[J].南京工业大学学报（自然科学版）,2011(06):20-25. |
| [36] | 朱兆连,孙敏,王海玲,张雪英,李爱民.垃圾渗滤液的Fenton氧化预处理研究[J].生态环境学报,2010(10):2484-2488. |
| [37] | 郭劲松,陈鹏,方芳,刘智萍,刘国强.Fenton试剂对垃圾渗滤液中有机物的去除特性研究[J].中国给水排水,2008(03):88-91. |
| [38] | 曹姝文,周林,肖晶.混凝-Fenton氧化法对晚期垃圾渗沥液有机物的去除特性研究[J].环境卫生工程,2012(05):37-38,43. |
| [39] | 吴彦瑜,覃芳慧,赖杨兰,彭华平,周少奇.Fenton试剂对垃圾渗滤液中腐殖酸的去除特性[J].环境科学研究,2010(01):94-99. |
| [40] | 丁辉,李鑫钢,徐世民.光助Fenton氧化垃圾渗滤液中腐殖质研究[J].太阳能学报,2008(06):761-766. |
| [41] | 周健,李宝霞,龙腾锐,林明波.微波强化Fenton氧化法处理垃圾渗滤液试验研究[J].中国给水排水,2009(17):97-99. |
| [42] | 肖书虎,宋永会,肖宏康,张国芳.以活性炭纤维为阴极的光电化学法协同处理垃圾渗滤液[J].环境工程技术学报,2011(04):353-358. |
| [43] | Moravia W G,Amaral M C S,Lange L C .Evaluation of landfill leachate treatment by advanced oxidative process by Fenton′s reagent combined with membrane separation system[J].Waste Management,2013,33 |
| [44] | Silva T F C V,Fonseca A,Saraiva I,et al .Biodegradability enhancement of a leachate after biological lagooing using a solar driven photo-Fenton reaction,and further combination with an activated sludge biological process,at pre-industrial scale[J].Water Research,2013,47(10):3543-3557. |
| [45] | Pillai K C,Kwon T O,Moon I S .Degradation of wastewater from terephthalic acid manufacturing process by ozonation catalyzed with Fe2+,H2 O2 and UV light:Direct versus indirect ozonation reaction[J].Applied Catalysis B:Environmental,2009,91 |
| [46] | 卢铭,李建明,陈志,梁希,彭辉.垃圾渗滤液的臭氧处理[J].四川环境,2005(06):40-44,49. |
| [47] | 宋世龙,张志强.基于臭氧氧化的垃圾渗沥液处理技术[J].环境卫生工程,2012(04):40-44. |
| [48] | 熊代群.臭氧强化光催化氧化处理渗滤液的研究[J].广东化工,2012(08):134-135,117. |
| [49] | 黄报远,金腊华,卢显妍,刘慧璇,唐崇杰.臭氧化对垃圾填埋场后期渗滤液的预处理研究[J].环境污染治理技术与设备,2006(04):103-106. |
| [50] | 沈小星,陈哲铭,方士,姚铭,王凯雄.老龄垃圾渗滤液混凝-催化臭氧氧化工艺研究[J].浙江大学学报（农业与生命科学版）,2006(04):449-454. |
| [51] | 刘卫华,季民,张昕,杨洁.催化臭氧氧化去除垃圾渗滤液中难降解有机物的研究[J].环境化学,2007(01):58-61. |
| [52] | 王苗苗 .光催化氧化技术对垃圾渗滤液深度处理的试验研究[D].天津大学,2007. |
| [53] | 梁梁,尹军,蒋宝军,吴晓燕.催化氧化技术处理垃圾渗滤液的研究进展[J].中国资源综合利用,2009(12):41-43. |
| [54] | 樊彩梅,孙彦平.纳米TiO2对水中腐殖酸的吸附及光催化降解[J].应用化学,2001(11):912-914. |
| [55] | Qazaq A S,Hudaya T,Lee I A L,et al .Decontamination of a natural multicomponent aqueous liquid waste by titania photocatalysis[J].International Journal of Environmental Technology and Management,2008,9 |
| [56] | Wiszniowski J,Robert D,Surmacz-Gorska J,et al .Leachate detoxification by combination of biological and TiO2-photocatalytic processes[J].Water Science & Technology,2006,53 |
| [57] | Renou S,Givaudan J G,Poulain S,et al .Landfill leachate treatment:Review and opportunity[J].Journal of Hazardous Materials,2008,150 |
| [58] | Poblete R,Otal E,Vilches L F,et al .Photocatalytic degradation of humic acids and landfill leachate using a solid industrial by-product containing TiO2 and Fe[J].Applied Catalysis B:Environmental,2011,102 |
| [59] | Oh S,Chiu P C,Kim B J,et al .Zero-valent iron pretreatment for enhancing the biodegradability of RDX[J].Water Research,2005,39(20):5027-5032. |
| [60] | 汤贵兰,蓝伟光,张烨,严滨,何旭敏,陈小强.焦炭和废铁屑微电解预处理垃圾渗滤液的研究[J].环境污染治理技术与设备,2006(11):121-123. |
| [61] | 谢武,潘琼,王金菊.催化型微电解对垃圾渗滤液深度处理的研究[J].西南农业学报,2011(05):1943-1947. |
| [62] | 赵剑锋,张宏伟.垃圾渗滤液脱氮处理工艺的工程实例[J].有色冶金设计与研究,2006(04):54-56,65. |
| [63] | 陈宏宇,孙宝盛.霸州市垃圾填埋场渗滤液处理工程设计与运行[J].水处理技术,2008(02):86-88,91. |
| [64] | 曹占平,张景丽,张宏伟.生化预处理-O3-MBR工艺在垃圾渗滤液处理中的应用[J].给水排水,2008(10):54-57. |
| [65] | 张璐,李武,高兴斋,刘芳佞,孙志军.垃圾焚烧发电厂渗滤液处理工程设计[J].中国给水排水,2009(04):29-31,34. |
| [66] | 孙志军,张璐,顾铮.预处理+生化+膜+臭氧工艺处理垃圾焚烧厂渗滤液[J].工业安全与环保,2010(06):48-50. |
| [67] | 杨拓 .汉沽垃圾填埋场渗滤液多级生化处理工艺的运行分析[D].天津大学,2007. |
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