欢迎登录材料期刊网

材料期刊网

中国科学院金属研究所 科学出版社
高级检索
  1. 首页
  2. 期刊
  3. 贵金属
  4. 富氧条件下烃类选择性催化还原NO用纳米贵金属催化剂的研究进展

贵金属, 2005, 26(4): 66-72. doi: 10.3969/j.issn.1004-0676.2005.04.014

富氧条件下烃类选择性催化还原NO用纳米贵金属催化剂的研究进展

田亚锋 1, , 吴军良 2, , 叶代启 3, , 付名利 4,

1.华南理工大学环境科学与工程学院,广东,广州,510640

2.华南理工大学环境科学与工程学院,广东,广州,510640

3.华南理工大学环境科学与工程学院,广东,广州,510640

4.华南理工大学环境科学与工程学院,广东,广州,510640

关键词： 催化化学 , 纳米贵金属催化剂 , 烃类 , 富氧 , NO , SCR

Research Progress on Nanometer Noble-metal Catalysts for the Selective Catalytic Reduction of NO by Hydrocarbon in the Presence of Excess Oxygen

纳米贵金属系列催化剂以其特有的性能得到广泛研究.本文对纳米贵金属催化剂(Pt、Pd、Rh、Ag、Ir、Au)在富氧条件下进行烃类选择性催化还原NO的性能、特点以及存在的问题进行了分析,介绍了复合贵金属催化剂体系及其反应机理,提出了对进一步改善纳米贵金属催化剂性能的途径.

参考文献

[1] Burch R;Anita Ramli .A comparative investigation of the reduction of NO by CH4 on Pt,Pd,and Rh catalysts[J].Applied Catalysis B:Environmental,1998,15:49-62.
[2] J.M.Garcia-Cortes;J.Perez-Ramirez;M.J.Illan-Gomez;F.Kapteijn;J.A.Moulijn;C.Salinas-Martinez de Lecea .Comparative study of Pt-based catalysts on different supports in the low-temperature de-NO_x-SCR with propene[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2001(3/4):399-408.
[3] Mariscal R;Rojas S;Gómez-Cortés A et al.Support effects in Pt/TiO2-ZrO2 catalysts for NO reduction with CH4[J].Catalysis Today,2002,75:385-391.
[4] Hanna Harelind Ingelsten;Magnus Skoglundh;Erik Fridell .Influence of the support acidity of Pt/aluminum-silicate catalysts on the continuous reduction of NO under lean conditions[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2003(3):287-300.
[5] Ning Li;Aiqin Wang;Lin Li;Xiaodong Wang;Lili Ren;Tao Zhang .NO reduction by CH_4 in the presence of excess O_2 over Pd/sulfated alumina catalysts[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2004(1):1-7.
[6] Consuelo Montes de Correa;Fernando Cordoba;Felipe Bustamante .The role of zeolite type on the lean NO_x rrduction by methane over Pd loaded pentasil zeolites[J].Microporous and Mesoporous Materials,2000(1/3):149-157.
[7] Shimizu Ken-ichi .Catalytic performance of Ag-Al_2O_3 catalyst for the selective catalytic reduction of NO by higher hydrocarbons[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2000(4):239-247.
[8] Yunbo Yu;Hong He;Qingcai Feng;Hongwei Gao;Xin Yang .Mechanism of the selective catalytic reduction of NO_x byC_2H_5OH over Ag/Al_2O_3[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2004(3):159-171.
[9] Shigeo Satokawa;Ken0ichi Yamaseki;Hiroshi Uchida .Influence of low concentation of SO_2 for selective reductin of NO by C_3H_8 in lean-exhaust conditiions on the activity of Ag/Al_2O_3 catalyst[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2001(4):299-306.
[10] Shigeo Satokawa;Junji Shibata;Ken-ichi Shimizu;Atsushi Satsuma;Tadashi Hattori .Promotion effect of H_2 on the low temperature activity of the selective reduction of NO by light hydrocarbons over Ag/Al_2O_3[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2003(2):179-186.
[11] Junji Shibata;Yuu Takada;Atsushi Satsuma;Tadashi Hattori;Shigeo Satokawa .Ag cluster as active species for SCR of NO by propane in the presence of hydrogen over Ag-MFI[J].Journal of Catalysis,2004(2):368-376.
[12] M.Richter;U.Bentrup;R.Eckelt;M.Schneider;M.-M.Pohl;R.Fricke .The effect of hydrogen on the selective catalytic reduction of NO in excess oxygen over Ag/Al_2O_3[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2004(4):261-274.
[13] C.Wogerbauer;M.Maciejewski;A.Baiker .Reduction of nitrogen oxides over unsupported iridium: effect of reducing agent[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2001(1):11-27.
[14] C.Wogerbauer;M.Maciejewski;A.Baiker .Structure sensitivity of NO reduction over iridium catalysts in HC-SCR[J].Journal of Catalysis,2002(1):157-167.
[15] C. Wogerbauer;M. Maciejewski;M.M. Schubert .Effect of sodium on the catalytic properties of iridium black in the selective reduction of NO_x by propene under lean-burn conditions[J].Catalysis Letters,2001(1/2):1-7.
[16] 周华,董守安.纳米金负载型催化剂的研究进展[J].贵金属,2004(02):48-56.
[17] Atsushi Ueda;Takeshi Oshima;Masatake Haruta .Reduction of nitrogen monoxide with propene in the presence of oxygen and moisture over gold supported on metal oxides[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,1997(2/3):81-93.
[18] Erol seker;John Cavataio;Erdogan Gulari;Paisan Lorpongpaiboon;Somchai Osuwan .Nitric oxide reduction by propene over silver/alumina and silver-gold/alumina catalysts:effect of preparation methods[J].Applied Catalysis, A. General: An International Journal Devoted to Catalytic Science and Its Applications,1999(1):121-134.
[19] 刘志明,郝吉明,朱天乐,傅立新.富氧条件下NOx催化净化的研究进展[J].环境污染治理技术与设备,2002(08):41-47.
[20] Hideaki Hamada .Cooperation of catalytic species for the selective reduction of nitrogen monoxide with hydrocar - bons[J].Catalysis Surveys from Japan,1997,1:53-60.
[21] Hirofumi Ohtsuka .The selective catalytic reduction of nitrogen oxides by methane on noble metal-loaded sulfated zirconia[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2001(4):325-333.
[22] Kazuhito Sato;Tomohiro Yoshinari;Yoshiaki Kintaichi;Masaki Haneda;Hideaki Hamada .Remarkable promoting effct of rhodium on the catalytic performance of Ag/Al_2O_3 for the selective reduciton of NO with decane[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2003(1):67-78.
[23] G.B.F.Seijger;P.van Kooten Niekerk;K.Krishna;H.P.A.Calis;H.van Bekkum;C.M.van den Bleek .Screening of silver and cerium exchanged zeolite catalysts for the lean burn reduction of NO_x with propene[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2003(1):31-42.
[24] Jeon JY.;Kim HY.;Woo SI. .Selective catalytic reduction of NOx in lean-burn engine exhaust over a Pt/V/MCM-41 catalyst[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2003(4):311-323.
[25] 李俊华,郝吉明,傅立新,朱天乐.富氧条件下选择性还原NO的复合催化剂体系[J].环境污染治理技术与设备,2003(09):1-6.
[26] Seker Erol;Gulari Erdogan .Activity and N_2 Selectivity of Sol-Gel Prepared Pt/Alumina Catalysts for Selective NO_x Reduction[J].Journal of Catalysis,2000(1):4-13.
[27] Nicolas Bion;Jacques Saussey;Masaaki Hanedeta et al.Study by in situ FTIR spectroscopy of the SCR of NOx by ethanol on Ag/Al2O3-evidence of the role of isocyanate species[J].Journal of Catalysis,2003,217:47-58.
[28] Piyasan Praserthdam;Choowong Chaisuk;Apiwat Panit;Kriangsak Kraiwattanawong .Some aspecs about the nature of surface species on Pt-based and MFI-based catalysts for the selective catalytic reduction of NO by propene under lean-burn condition[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2002(3):227-241.
[29] Joel Despres;Martin Elsener;Manfred Koebel .Catalytic oxidation of nitrogen monoxide over Pt/SiO_2[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2004(2):73-82.
[30] Michael J Kirkpatrick;Wright C Finney;Bruce R Locke .Plasma-catalyst interactions in the treatment of volatile organic compounds and NOx with pulsed corona discharge and reticulated vitreous carbon Pt/Rh- coated electrodes[J].Catalysis Today,2004,89:117-126.
上一张 下一张
上一张 下一张
计量
  • 下载量()
  • 访问量()
作者相关
文章评分
  • 您的评分：
  • 1
    0%
  • 2
    0%
  • 3
    0%
  • 4
    0%
  • 5
    0%

版权所有©2010中国科学院金属研究所中国科技出版传媒股份有限公司

本系统由北京仁和汇智信息技术有限公司设计开发

技术支持：info@rhhz.net