金属-载体强相互作用(SMSI)的发生机理及其对催化活性的影响是目前CeO2基三效催化剂研究的热点.介绍了金属-载体强相互作用产生的基本条件及其基本特征,综述了贵金属与CeO2基复合氧化物间SMSI的可能机制及相关研究进展,提出了金属-载体强相互作用可能的研究方向.
参考文献
[1] | Tauster S J;Fung S C;Garten R L .Strong metal-suppert interactions.Group 8 noble metals supperted on titanium dioxide[J].Journal of the American Chemical Society,1978,100:170-175. |
[2] | Abid M;Paul-Boncour V;Touroude R .Pt/CeO2 catalysts in crotonaldehyde hydrogenation: Selectivity, metal particle size and SMSI states[J].Applied Catalysis, A. General: An International Journal Devoted to Catalytic Science and Its Applications,2006(1):48-59. |
[3] | 张敏,金振声,张治军,党鸿辛.金属-载体强相互作用及其对多相催化反应的影响[J].河南大学学报(自然科学版),2005(04):21-26. |
[4] | 游少雄,冯长根,王丽琼,曾庆轩,安琴,王亚军.催化剂Pd/CeO2中Pd 与 CeO2之间的SMSI对汽车尾气的催化活性的影响[J].化工科技,2001(03):20-23. |
[5] | Tauster S J;Fung S C .Strong metal-support interaction:Occurrence among the binary oxides of group ⅡA-ⅡB[J].Journal of Catalysis,1978,55:29-35. |
[6] | Bozo C;Guilhaume N;Herrmann J-Marie .Role of the ceria-zirconia support in the reactivity of platinum and palladium catalysts for methane[J].Journal of Catalysis,2001,203:393-406. |
[7] | Bernal S;Calvino J J;Cauqui M A et al.Some recent results on metal/support interaction effects in NM/CeO2(NM:noble metal)catalysts[J].Catalysis Today,1999,50:175-206. |
[8] | L.F.Liotta;A.Longo;A.Macaluso;A.Martorana;G.Pantaleo;A.M.Venezia;G.Deganello .Influence of the SMSI effect on the catalytic activity of a Pt(1%)/Ce_(0.6)Zr_(0.4)O_2 catalyst:SAXS,XRD,XPS and TPR investigations[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2004(2):133-149. |
[9] | L.Osterlund;S.Kielbassa;C.Werdinius;B.Kasemo .Reactivity of Pt/ceria and Pt/alumina planar model catalysts prepared by colloidal lithography[J].Journal of Catalysis,2003(1):94-107. |
[10] | Yao Y F Yu .The oxidation of CO and hydrocarbons over noble metal catalysts[J].Journal of Catalysis,1984,87:152-162. |
[11] | Nunan J G;Robots H J;Cohn M J et al.Physico-chemical properties of Ce-containing three-way catalysts and the effect of Ce on catalyst activity[J].Journal of Catalysis,1992,133:309-324. |
[12] | Stanislaw E. Golunski;Helen A. Hatcher;Raj R. Rajaram;Timothy J. Truex .Origins of low-temperature three-way activity in Pt/CeO_2[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,1995(4):367-376. |
[13] | Diwell A F;Rajaram R R;Shaw H A.Catalysis and automotive pellution control Ⅱ.Studies in surface science and catalysis[M].Amsterdam:Elsevier Science,1991:139. |
[14] | Serre C;Garin F;Belot G;Maire G .Reactivity of Pt/Al2O3 and Pt-CeO2Al2O3 catalysts for the oxidation of carbon monoxide by oxygen:Ⅱ.Influence of the pretreatment step on the oxidation mechanism[J].Journal of Catalysis,1993,141:9-20. |
[15] | Anna Holmgren;Fazlollah Azarnoush;Erik Fridell .Influence of pre-treatment on the low-temperature activity of Pt/ceria[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,1999(1):49-61. |
[16] | Fan J;Wu XD;Ran R;Weng DA .Influence of the oxidative/reductive treatments on the activity of Pt/Ce0.67Zr0.33O2 catalyst[J].Applied Surface Science: A Journal Devoted to the Properties of Interfaces in Relation to the Synthesis and Behaviour of Materials,2005(1/4):162-171. |
[17] | Sanchez M G;Gazquez J L .Oxygen vacancy model in strong metal-suppert interaction[J].Journal of Catalysis,1987,104:120-135. |
[18] | Nagai Y;Hirabayashi T;Dohmae K et al.Sintering inhibition mechanism of platinum supperted on ceria-based oxide and Pt-oxide-suppert interaction[J].Journal of Catalysis,2006,242:103-109. |
[19] | Frost J C .Junction effect interactions in methanol synthesis catalysts[J].Nature,1988,334:577-580. |
[20] | Graham G.W.;Jen H.-W.;Chun W. .High-Temperature-Aging-Induced Encapsulation of Metal Particles by Support Materials: Comparative Results for Pt, Pd, and Rh on cerium-Zirconium Mixed Oxides[J].Journal of Catalysis,1999(1):228-233. |
[21] | Naito S;Kasahara T;Miyao T .Transformation of methane formation sites into methanol formation ones duringCO-H2 reaction over Pd/CeO2 in its SMSI state[J].Catalysis Today,2002,74:201-206. |
[22] | Bernal S;Botana F J;Calvino J J et al.HREM study of the behaviour of a Rh/CeO2 catalyst under high temperature reducing and oxidizing conditions[J].Catalysis Today,1995,23:219-250. |
[23] | Bernal S;Cauqui M A;Cifredo G A et al.Chemical and microstructural investigation of Pt/CeO2 catalysts reduced at temperatures ranging from 473 to 973K[J].Catalysis Today,1996,29:77-81. |
[24] | Kepinski L;Wolcyrz M;Okal J .Effect of chlorine on microstracture and activity of Pd/CeO2 catalyst[J].Journal of the Chemical Society,Faraday Transactions,1995,91(03):507-515. |
[25] | Jun Fan;Xiaodong Wu;Xiaodi Wu .Thermal ageing of Pt on low-surface-area CeO2-ZrO2-La2O3 mixed oxides: Effect on the OSC performance[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2008(1/2):38-48. |
[26] | Hardacre C.;Lambert RM.;Rayment T. .PLATINUM/CERIA CO OXIDATION CATALYSTS DERIVED FROM PT/CE CRYSTALLINE ALLOY PRECURSORS[J].Journal of Catalysis,1996(1):102-108. |
[27] | Penner S.;Wang D.;Su DS.;Rupprechter G.;Podloucky R.;Schlogl R. Hayek K. .Platinum nanocrystals supported by silica, alumina and ceria: metal-support interaction due to high-temperature reduction in hydrogen[J].Surface Science: A Journal Devoted to the Physics and Chemistry of Interfaces,2003(0):276-280. |
[28] | Bernal S.;Gatica JM.;Larese C.;Lopezcartes C.;Perezomil JA.;Calvino JJ. .NANOSTRUCTURAL EVOLUTION OF A PT/CEO2 CATALYST REDUCED AT INCREASING TEMPERATURES (473-1223 K) - A HREM STUDY[J].Journal of Catalysis,1997(2):510-515. |
[29] | Penner S.;Rupprechter G.;Sauer H.;Su DS.;Tessadri R.;Podloucky R. Schlogl R.;Hayek K. .Pt/ceria thin film model catalysts after high-temperature reduction: a (HR)TEM study[J].Vacuum: Technology Applications & Ion Physics: The International Journal & Abstracting Service for Vacuum Science & Technology,2003(1/2):71-76. |
[30] | Kepi(n)ski L;Wolcyrz M .Microstructure of Pd/CeO2 catalyst:Effect of high temperature reduction in hydrogen[J].Applied Catalysis A:General,1997,150:197-220. |
上一张
下一张
上一张
下一张
计量
- 下载量()
- 访问量()
文章评分
- 您的评分:
-
10%
-
20%
-
30%
-
40%
-
50%