首次将钙钛石 BiMnO3用于低温条件下 NH3选择性催化还原 NO 反应中.结果表明,该催化剂在100~240 oC 范围内表现出较好的催化活性.实验和理论计算显示,相对于 LaMnO3, BiMnO3优异的低温催化活性归因于其较强的 Lewis 酸性和较多的表面吸附氧物种.此外, BiMnO3还具有较好的抗水、抗硫性能.
参考文献
| [1] | Busca G;Lietti L;Ramis G;Berti F .[J].Applied Catalysis B:Environmental,1998,18:1. |
| [2] | Li J;Chang H;Ma L;Hao J Yang R T .[J].Catalysis Today,2011,175:147. |
| [3] | Smirniotis P G;Pena D A;Uphade B S .[J].Angewandte Chemie International Edition,2001,40:2479. |
| [4] | Qi G;Yang R T.[J].Chemical Communications,2003:848. |
| [5] | Chen, Z.;Yang, Q.;Li, H.;Li, X.;Wang, L.;Chi Tsang, S. .Cr-MnO_x mixed-oxide catalysts for selective catalytic reduction of NO_x with NH_3 at low temperature[J].Journal of Catalysis,2010(1):56-65. |
| [6] | Liu F;He H .[J].Catalysis Today,2010,153:70. |
| [7] | Yang S;Wang C;Li J;Yan N Ma L Chang H .[J].Applied Catalysis B:Environmental,2011,110:71. |
| [8] | 唐幸福,李俊华,魏丽斯,郝吉明.氧化还原沉淀法制备MnOx-SnO2催化剂及其对NO的NH3选择催化还原性能[J].催化学报,2008(06):531-536. |
| [9] | Pena M A;Fierro J L G .[J].Chemical Reviews,2001,101:1981. |
| [10] | Viswanathan B .[J].Catalysis Review:Science and Engineering,1992,34:337. |
| [11] | Seiyama T .[J].Catalysis Review:Science and Engineering,1992,34:281. |
| [12] | Voorhoeve R J H;Johnson D W;Remeika J P;Gallagher P K .[J].Science,1977,195:827. |
| [13] | Kim C H;Qi G;Dahlberg K;Li W .[J].Science,2010,327:1624. |
| [14] | Zhu J;Thomas A .[J].Applied Catalysis B:Environmental,2009,92:225. |
| [15] | Tops?e N Y .[J].Science,1994,265:1217. |
| [16] | Li, Y;Cheng, H;Li, DY;Qin, YS;Xie, YM;Wang, SD .WO3/CeO2-ZrO2, a promising catalyst for selective catalytic reduction (SCR) of NOx with NH3 in diesel exhaust[J].Chemical Communications,2008(12):1470-1472. |
| [17] | 李飞,肖德海,张一波,王德强,潘喜强,杨向光.用于NH3选择催化还原NO反应的新型Ce-P-O催化剂[J].催化学报,2010(08):938-942. |
| [18] | Li F;Zhang Y B;Xiao D H;Wang D Q Pan X Q Yang X G .[J].ChemCatChem,2010,2:1416. |
| [19] | Samuel V;Navale S C;Jadhav A D;Gaikwad A B Ravi V .[J].Materials Letters,2007,61:1050. |
| [20] | 姚长达,巩江峰,耿芳芳,高虹,徐云玲,张爱梅,唐春梅,朱卫华.常温常压下BiMnO3纳米粉末的制备与物性分析[J].物理学报,2010(08):5332-5337. |
| [21] | Zhu J J;Xiao D H;Li J J;Yang X G .[J].Catalysis Letters,2009,129:240. |
| [22] | Kapteijn F;Singoredjo L;Andreini A;Moulijn J A .[J].Applied Catalysis B:Environmental,1994,3:173. |
| [23] | Chuah G K;Liu S H;Jaenicke S;Harrison L J .[J].Journal of Catalysis,2001,200:352. |
| [24] | Kijlstra WS.;Poels EK.;Bliek A.;Brands DS. .MECHANISM OF THE SELECTIVE CATALYTIC REDUCTION OF NO BY NH3 OVER MNOX/AL2O3 .1. ADSORPTION AND DESORPTION OF THE SINGLE REACTION COMPONENTS[J].Journal of Catalysis,1997(1):208-218. |
| [25] | Jeong N C;Lee J S;Tae E L;Lee Y J,Yoon K B .[J].Angewandte Chemie International Edition,2008,47:10128. |
| [26] | Sanderson R T .[J].Science,1951,114:670. |
| [27] | Jacobs P A;Mortier W J;Uytterhoeven J B .[J].Journal of Inorganic and Nuclear Chemistry,1978,40:1919. |
| [28] | Karazhanov, SZ;Ravindran, P .Ab Initio Study Of Double Oxides ZnX_2O_4 (X=Al, Ga, In) Having Spinel Structure[J].Journal of the American Ceramic Society,2010(10):3335-3341. |
| [29] | Du J;Corrales L R .[J].Journal of Physical Chemistry B,2006,110:22346. |
| [30] | Kang M;Park E D;Kim J M;Yie J E .[J].Applied Catalysis A:General,2007,327:261. |
| [31] | Heidler R;Janssens G O A;Mortier W J;Schoonheydt R A .[J].Journal of Physical Chemistry,1996,100:19728. |
| [32] | Koebel M;Madia G;Elsener M .[J].Catalysis Today,2002,73:239. |
| [33] | Zhang Q;Qiu C;Xu H;Lin T Lin Z Gong M Chen Y .[J].Catalysis Today,2011,175:171. |
上一张
下一张
上一张
下一张
计量
- 下载量()
- 访问量()
文章评分
- 您的评分：
-
10%
-
20%
-
30%
-
40%
-
50%